Subnanosecond X-ray diffraction technique for studying laser-induced polarization-dependent processes in KISI-Kurchatov

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The dynamics of the diffraction peak 0012 parameters of LiNbO3:Fe crystals with a time resolution of less than 1 ns were recorded by synchronizing nanosecond laser pulses with electron bunches of the KISI-Kurchatov synchrotron source. The influence of a laser pulse (λ = 532 nm, t = 4 ns, energy density 0.6 J/cm2) at different polarization directions of the laser radiation causes a change in the peak intensity, which depends on the angle between the polarization direction of the laser radiation and the crystallographic axes. The obtained results are supplemented with wavelet analysis of experimental data. The observed polarization dependence correlates with published data on the photovoltaic effect.

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作者简介

M. Kovalchuk

Shubnikov Institute of Crystallography of Kurchatov Complex of Crystallography and Photonics of NRC “Kurchatov Institute”

Email: mareev.evgeniy@physics.msu.ru
俄罗斯联邦, Moscow

E. Mareev

Shubnikov Institute of Crystallography of Kurchatov Complex of Crystallography and Photonics of NRC “Kurchatov Institute”

编辑信件的主要联系方式.
Email: mareev.evgeniy@physics.msu.ru
俄罗斯联邦, Moscow

A. Kulikov

Shubnikov Institute of Crystallography of Kurchatov Complex of Crystallography and Photonics of NRC “Kurchatov Institute”

Email: ontonic@gmail.com
俄罗斯联邦, Moscow

F. Pilyak

Shubnikov Institute of Crystallography of Kurchatov Complex of Crystallography and Photonics of NRC “Kurchatov Institute”

Email: mareev.evgeniy@physics.msu.ru
俄罗斯联邦, Moscow

N. Obydennov

Shubnikov Institute of Crystallography of Kurchatov Complex of Crystallography and Photonics of NRC “Kurchatov Institute”; Lomonosov Moscow State University

Email: mareev.evgeniy@physics.msu.ru
俄罗斯联邦, Moscow; Moscow

F. Potyomkin

Lomonosov Moscow State University

Email: mareev.evgeniy@physics.msu.ru
俄罗斯联邦, Moscow

Yu. Pisarevsky

Shubnikov Institute of Crystallography of Kurchatov Complex of Crystallography and Photonics of NRC “Kurchatov Institute”

Email: mareev.evgeniy@physics.msu.ru
俄罗斯联邦, Moscow

N. Marchenkov

Shubnikov Institute of Crystallography of Kurchatov Complex of Crystallography and Photonics of NRC “Kurchatov Institute”

Email: mareev.evgeniy@physics.msu.ru
俄罗斯联邦, Moscow

A. Blagov

Shubnikov Institute of Crystallography of Kurchatov Complex of Crystallography and Photonics of NRC “Kurchatov Institute”

Email: mareev.evgeniy@physics.msu.ru
俄罗斯联邦, Moscow

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2. Fig. 1. Time range of some physical processes that can be registered at different X-ray sources

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3. Fig. 2. Schematic diagram of the experimental setup: BM - SI source (rotating magnet), Slits1 - white beam slits, Slits2 - monochromatized beam slits, M - Si 111 dual crystal monochromator, IC - ionization chamber, G - goniometer with a mounted sample, S - sample, L - laser radiation source, D - deflector, PG - Glahn prism. The synchronization board triggers the laser control unit with a preset delay according to the reference high-frequency signal of the storage ring. The oscilloscope allows to digitize the analog signal coming from the detector

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4. Fig. 3. BWC dynamics of LiNbO3:Fe crystal (reflex 0012) under laser pulse exposure (white dashed line indicates the initial moment of exposure) for different azimuthal angles φ coinciding with the direction of laser radiation polarization relative to the crystallographic axis X [20]. The results are plotted as three-dimensional maps (color indicates the intensity of the registered signal at a given time delay and angular position). The value of the angle φ is indicated in the upper right corner

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5. Fig. 4. Three-dimensional visualization of wavelet analysis of data for azimuth angles of 0° and 120°

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